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Author
Kiang, J. K. Y. | Uden, P. C. | Chien, J. C. W.
Title
Polymer Reactions. Part 7. Thermal Pyrolysis of Poly(Isoprene).
Coporate
Massachusetts Univ., Amherst
Sponsor
National Institute of Standards and Technology, Gaithersburg, MD
Report
Part 7
no date
27 p.
Contract
NBS-GRANT-G7-9010
Keywords
pyrolysis | polypropylene | flash pyrolysis
Abstract
Poly(propylene) has been pyrolyzed in a carrier stream of helium from 388 deg to 900 deg C in both programmed heating and flash pyrolysis modes. The products were on-line identified and quantitatively analyzed by an interfaced GC peak identification system. The first order rate constants for pyrolysis are 3.7 x 10(-4) sec.(-1) and 4.0 x 10(-4) sec.(-1), respectively, for atactic and isotactic poly(propylene) at 388 deg C; the corresponding overall activation energies are 56 ±6 and 51 ±5 kcal. mole(-1). The main products in decreasing yields are 2,4-dimethyl-l-heptene, 2-pentene, propylene, 2 methyl-l-pentene, and 2,4,6-trimethyl-l-nonene.