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Author
Gilman, J. W. | Bourbigot, S. | Shields, J. R. | Nyden, M. R. | Kashiwagi, T. | Davis, R. D. | Vanderhart, D. L. | Demory, W. | Wilkie, C. A. | Morgan, A. B. | Harris, J. | Lyon, R. E.
Title
High Throughput Methods for Polymer Nanocomposites Research: Extrusion, NMR Characterization and Flammability Property Screening.
Coporate
National Institute of Standards and Technology, Gaithersburg, MD GEMTEX, Roubaix, France Marquette Univ., Milwaukee, WI Dow Chemical Corp., Midland, MI Federal Aviation Administration Technical Center, Atlantic City, NJ
Journal
Journal of Materials Science, Vol. 38, 4451-4460, 2003
Keywords
nanocomposites | flammability | cone calorimeters | polymers
Identifiers
Transmission Electron Microscopy (TEM); NMR
Abstract
A large number of parameters influence polymer-nanocomposite performance and developing a detailed understanding of these materials involves investigation of a large volume of the associated multi-dimensional property space. This multi-dimensional parameter space for polymer-nanocomposites consists of the obvious list of different material types under consideration, such as polymer and nano-additive, but also includes interphase surface chemistry, and processing conditions. This article presents combinatorial library design and high-throughput screening methods for polymer nanocomposites intended as flame-resistant materials. Here, we present the results of using a twin-screwn extruder to create composition-gradient library strips of polymer nanocomposites that are screened with a solid-state NMR method to rapidly evaluate the optimal processing conditions for achieving nanocomposite dispersion. In addition, we present a comparison of a new rapid Cone calorimetry method to conventional Cone calorimetry and to the gradient heat-flux flame spread method.